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CO2还原光催化材料研究进展

Research Progress in Photocatalytic Materials for CO2 Reduction

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【作者】 许丹于彩莲李芬杨莹李博琳芦柳蔺宇晨

【Author】 XU Dan;YU Cailian;LI Fen;YANG Ying;LI Bolin;LU Liu;LIN Yuchen;School of Materials Science and Chemical Engineering, Harbin University of Science and Technology;

【通讯作者】 于彩莲;

【机构】 哈尔滨理工大学材料科学与化学工程学院

【摘要】 太阳能驱动二氧化碳转化为可持续的碳氢燃料是缓解能源危机和全球气候变暖问题的一条重要战略途径。选择高效且经济的光催化材料是实现光催化CO2转化为高附加值产物的关键。本文主要从光催化CO2还原反应机理、催化剂类型等方面综述了光催化CO2还原领域的研究进展,着重讨论了光催化剂改性策略,包括构筑异质结、金属掺杂、形貌调控等。目前,选择合适高效的光催化材料用以光催化CO2还原制备高附加值产物等方面尚存在些许不足,比如光催化CO2转化效率低、产物选择性差以及无法规模化投入生产等问题,因此如何解决上述问题是未来光催化CO2资源化领域的研究重点。

【Abstract】 One meaningful and strategic way to alleviate the energy crisis and global warming issues is to use hydrocarbon fuels converted using solar energy from carbon dioxide(CO2). Choosing efficient and economical photocatalytic materials is the key to obtaining high-value-added products from photocatalytic CO2. In this article, we aim to review the research progress in the field of photocatalytic CO2 reduction reactions from two perspectives: reaction mechanisms and catalyst types. Emphasis is placed on the discussion of photocatalyst modification methods, including constructing hereto-junctions, metal doping, and morphology regulation. However, selecting suitable and efficient photocatalytic materials for producing high-value-added products needs to be improved. We have problems such as low CO2 conversion efficiency, poor selectivity of products obtained, and inability to scale up production, therefore, how to solve these problems is the focus of research in the photocatalytic CO2 reduction field in the future.

【基金】 国家自然科学基金(22278100)~~
  • 【文献出处】 材料导报 ,Materials Reports , 编辑部邮箱 ,2024年14期
  • 【分类号】O643.36;O644.1
  • 【下载频次】143
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